Search results for "Entrance channel"
showing 3 items of 3 documents
Fission and quasifission of composite systems with Z=108−120 : Transition from heavy-ion reactions involving S and Ca to Ti and Ni ions
2016
Background: Suppression of compound nucleus formation in the reactions with heavy ions by a quasifission process in dependence on the reaction entrance channel.
Investigation of the reaction 64Ni+238U being an option of synthesizing element 120
2010
This study is concerned with the search for entrance channels suitable to synthesize elements with Z > 118. Mass-energy distributions as well as capture cross-sections of fission-like fragments have been measured for the reactions 64Ni + 238U → 302120 and 48Ca + 238U → 286112 at energies near the Coulomb barrier. Compound nucleus fission cross-sections were estimated from the analysis of mass and total kinetic energy distributions. The cross-section drops three orders of magnitude for the formation of the compound nucleus with Z = 120 obtained in the reaction 64Ni + 238U compared to the formation of the compound nucleus with Z = 112 obtained in the reaction 48Ca + 238U at an excitation ener…
Towards a converged barrier height for the entrance channel transition state of the N(2D)+CH4 reaction and its implication for the chemistry in Titan…
2011
Abstract The N( 2 D) + CH 4 reaction appears to be a key reaction for the chemistry of Titan’s atmosphere, opening the door to nitrile formation as recently observed by the Cassini–Huygens mission. Faced to the controversy concerning the existence or not of a potential barrier for this reaction, we have carried out accurate ab initio calculations by means of multi-state multi-reference configuration interaction (MS-MR-SDCI) method. These calculations have been partially corrected for the size-consistency errors (SCE) by Davidson, Pople or AQCC corrections. We suggest a barrier height of 3.86 ± 0.84 kJ/mol, including ZPE, for the entrance transition state, in good agreement with the experime…